Journal de Physique

Functionalizing Polymer Surfaces by Field-Induced Migration of Copolymer Additives. 1. Role of Surface Energy Gradients

Hojun Lee and Lynden A. Archer
Macromolecules 34 (13) 4572 (2001)
https://doi.org/10.1021/ma001278e

Surface Enrichment in Polymer Blends Involving Hydrogen Bonding

Yuzhi Duan, Eli M. Pearce, T. K. Kwei, et al.
Macromolecules 34 (19) 6761 (2001)
https://doi.org/10.1021/ma002093a

Polymer blends near patterned surfaces

Chaok Seok, Karl F. Freed and Igal Szleifer
The Journal of Chemical Physics 112 (14) 6452 (2000)
https://doi.org/10.1063/1.481276

SANS Study of Sulfonate End Group Effect on Polystyrene Self-Diffusion

S. D. Kim, A. Klein, L. H. Sperling, E. M. Boczar and B. J. Bauer
Macromolecules 33 (22) 8334 (2000)
https://doi.org/10.1021/ma000432u

Kirk-Othmer Encyclopedia of Chemical Technology

Dwain M. White
Kirk-Othmer Encyclopedia of Chemical Technology (2000)
https://doi.org/10.1002/0471238961.0118151323080920.a01

Phase separation in thin films of polymer blends: The influence of symmetric boundary conditions

Michael Wendlandt, Tobias Kerle, Marcus Heuberger and Jacob Klein
Journal of Polymer Science Part B: Polymer Physics 38 (6) 831 (2000)
https://doi.org/10.1002/(SICI)1099-0488(20000315)38:6<831::AID-POLB3>3.0.CO;2-P

Spatial and Temporal Dependence of Diffusion in Polystyrene Thin Films on Silicon and Carbon Surfaces

Y Strzhemechny, V Zaitsev, K Zhou, S A Schwarz, J Sokolov and M H Rafailovich
High Performance Polymers 12 (4) 611 (2000)
https://doi.org/10.1088/0954-0083/12/4/317

APPLICATIONS OF X-RAY PHOTOELECTRON SPECTROSCOPY AND STATIC SECONDARY ION MASS SPECTROMETRY IN SURFACE CHARACTERIZATION OF COPOLYMERS AND POLYMERS BLENDS

Chi-Ming Chan and Lu-Tao Weng
Reviews in Chemical Engineering 16 (4) (2000)
https://doi.org/10.1515/REVCE.2000.16.4.341

COMPUTER SIMULATION OF PROFILES OF INTERFACES BETWEEN COEXISTING PHASES: DO WE UNDERSTAND THEIR FINITE SIZE EFFECTS?

KURT BINDER and MARCUS MÜLLER
International Journal of Modern Physics C 11 (06) 1093 (2000)
https://doi.org/10.1142/S012918310000095X

Resonance enhancement of x rays in layered materials: Application to surface enrichment in polymer blends

B. N. Dev, Amal K. Das, S. Dev, et al.
Physical Review B 61 (12) 8462 (2000)
https://doi.org/10.1103/PhysRevB.61.8462

Determination of the interaction force between two adsorptive surfaces delimiting a critical binary polymer blend

A. Saout-Elhak, R. Cherrabi, M. Benhamou and M. Daoud
Physical Review E 62 (5) 6795 (2000)
https://doi.org/10.1103/PhysRevE.62.6795

Symmetric polymer blend confined into a film with antisymmetric surfaces: Interplay between wetting behavior and the phase diagram

M. Müller, E. V. Albano and K. Binder
Physical Review E 62 (4) 5281 (2000)
https://doi.org/10.1103/PhysRevE.62.5281

Surface segregation from polystyrene networks

Mark Geoghegan, François Boué, Alain Menelle, et al.
Journal of Physics: Condensed Matter 12 (24) 5129 (2000)
https://doi.org/10.1088/0953-8984/12/24/305

Wetting in a phase separating polymer blend film: Quench depth dependence

Mark Geoghegan, Hubert Ermer, Gerald Jüngst, Georg Krausch and Rüdiger Brenn
Physical Review E 62 (1) 940 (2000)
https://doi.org/10.1103/PhysRevE.62.940

Composition profiling in a binary polymer blend thin film using polarized neutron reflectivity

H Grüll, A Schreyer, N. F Berk, C. F Majkrzak and C. C Han
Europhysics Letters (EPL) 50 (1) 107 (2000)
https://doi.org/10.1209/epl/i2000-00242-8

Polymer melts and polymer solutions near patterned surfaces

Chaok Seok, Karl F. Freed and Igal Szleifer
The Journal of Chemical Physics 112 (14) 6443 (2000)
https://doi.org/10.1063/1.481206

Effect of Surface Segregation of Ionic End Groups on Polystyrene Latex Early-Time Interdiffusion

S. D. Kim, E. M. Boczar, A. Klein and L. H. Sperling
Langmuir 16 (3) 1279 (2000)
https://doi.org/10.1021/la990709n

Segmental Interaction Parameters of Binary Polymer Mixtures Evaluated from Binodals and from Surface-Segregation Profiles: Comparison with Small-Angle Neutron Scattering

Jacob Klein, Tobias Kerle, Florian Zink and Erika Eiser
Macromolecules 33 (4) 1298 (2000)
https://doi.org/10.1021/ma990798a

Wetting transition in a binary polymer blend

J Rysz, A Budkowski, A Bernasik, et al.
Europhysics Letters (EPL) 50 (1) 35 (2000)
https://doi.org/10.1209/epl/i2000-00231-y

Anisochemical Homopolymer/Diblock Copolymer Thin Film Blends

Michael D. Smith, Peter F. Green and Randall Saunders
Macromolecules 32 (25) 8392 (1999)
https://doi.org/10.1021/ma9908494

Surface Enrichment in a Miscible Random Copolymer Blend: Influence of Polydispersity and Architecture

Robert Oslanec, Jan Genzer, Alessandro Faldi, Russell J. Composto and Paul D. Garrett
Macromolecules 32 (12) 4098 (1999)
https://doi.org/10.1021/ma980601z

Chain conformation in ultrathin polymer films

Ronald L. Jones, Sanat K. Kumar, Derek L. Ho, Robert M. Briber and Thomas P. Russell
Nature 400 (6740) 146 (1999)
https://doi.org/10.1038/22080

Spinodal Decomposition in a Subsurface Layer of a Polymer Blend Film

Jakob Heier, Edward J. Kramer, Peter Revesz, Gabor Battistig and Frank S. Bates
Macromolecules 32 (11) 3758 (1999)
https://doi.org/10.1021/ma981709h

Polymers in Confined Environments

K. Binder
Advances in Polymer Science, Polymers in Confined Environments 138 1 (1999)
https://doi.org/10.1007/3-540-69711-X_1

Phase separation in confined polymer blends

R. Cherrabi, A. Saout-Elhak, M. Benhamou and M. Daoud
The Journal of Chemical Physics 111 (17) 8174 (1999)
https://doi.org/10.1063/1.480151

Interfaces Crystallization Viscoelasticity

Andrzej Budkowski
Advances in Polymer Science, Interfaces Crystallization Viscoelasticity 148 1 (1999)
https://doi.org/10.1007/3-540-48836-7_1

Surface Segregation of the Higher Surface Free Energy Component in Symmetric Polymer Blend Films

Tisato Kajiyama, Keiji Tanaka and Atsushi Takahara
Macromolecules 31 (11) 3746 (1998)
https://doi.org/10.1021/ma971247s

Surface studies of poly(methyl methacrylate)/poly(styrene-co-acrylonitrile) blends

Jacek M PigŁowski and Marek Bryjak
European Polymer Journal 34 (11) 1669 (1998)
https://doi.org/10.1016/S0014-3057(98)00023-8

Near-Surface Composition Profiles in Isotopic Polymer Blends Determined via High-Resolution Nuclear Reaction Analysis

Florian Zink, Tobias Kerle and Jacob Klein
Macromolecules 31 (2) 417 (1998)
https://doi.org/10.1021/ma970380h

High resolution elastic recoil detection analysis of polystyrene depth profiles using carbon ions

Mark Geoghegan and François Abel
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms 143 (3) 371 (1998)
https://doi.org/10.1016/S0168-583X(98)00344-9

Surface Molecular Aggregation Structure and Surface Molecular Motions of High-Molecular-Weight Polystyrene/Low-Molecular-Weight Poly(methyl methacrylate) Blend Films

Keiji Tanaka, Atsushi Takahara and Tisato Kajiyama
Macromolecules 31 (3) 863 (1998)
https://doi.org/10.1021/ma9709866

Wetting and Capillary Condensation in Symmetric Polymer Blends: A Comparison between Monte Carlo Simulations and Self-Consistent Field Calculations

M. Müller and K. Binder
Macromolecules 31 (23) 8323 (1998)
https://doi.org/10.1021/ma980052x

Surface enrichment and surface tension of oligo(styrene)/oligo(dimethylsiloxane) blends near the critical temperature

Takuhei Nose and Naoe Kasemura
Polymer 39 (24) 6137 (1998)
https://doi.org/10.1016/S0032-3861(98)00105-0

Surface enrichment-depletion duality in a binary polymer blend

A Budkowski, J Rysz, F Scheffold and J Klein
Europhysics Letters (EPL) 43 (4) 404 (1998)
https://doi.org/10.1209/epl/i1998-00373-4

Theoretical study of the prewetting transition in polymer blends

Gerald G. Pereira
The Journal of Chemical Physics 106 (10) 4282 (1997)
https://doi.org/10.1063/1.473130

Surface Enrichment from a Binary Polymer Blend

Ioannis G. Kokkinos and Marios K. Kosmas
Macromolecules 30 (3) 577 (1997)
https://doi.org/10.1021/ma960567t

New statistical mechanical treatment of systems near surfaces. I. Theory and principles

P. D. Gujrati and Mukesh Chhajer
The Journal of Chemical Physics 106 (13) 5599 (1997)
https://doi.org/10.1063/1.473600

Equilibrium concentration profiles of physically end tethered polystyrene molecules at the air-polymer interface

I. Hopkinson, F.T. Kiff, R.W. Richards, D.G. Bucknall and A.S. Clough
Polymer 38 (1) 87 (1997)
https://doi.org/10.1016/S0032-3861(96)00482-X

Critical Point Wetting for Binary Two-Phase Polymer−Solvent Mixtures on Solid Interfaces

F. A. M. Leermakers, L. J. M. Schlangen and L. K. Koopal
Langmuir 13 (21) 5751 (1997)
https://doi.org/10.1021/la9702704

Anomalous size-dependence of interfacial profiles between coexisting phases of polymer mixtures in thin-film geometry: A Monte Carlo simulation

Andreas Werner, Friederike Schmid, Marcus Müller and Kurt Binder
The Journal of Chemical Physics 107 (19) 8175 (1997)
https://doi.org/10.1063/1.475118

Surface phase behavior in binary polymer mixtures. III. Temperature dependence of surface enrichment and of wetting

A. Budkowski, F. Scheffold, J. Klein and L. J. Fetters
The Journal of Chemical Physics 106 (2) 719 (1997)
https://doi.org/10.1063/1.473407

Kinetics of Surface Segregation and the Approach to Wetting in an Isotopic Polymer Blend

M. Geoghegan, T. Nicolai, J. Penfold and R. A. L. Jones
Macromolecules 30 (14) 4220 (1997)
https://doi.org/10.1021/ma9603948

Surface segregation amplification in miscible polymer blends near criticality

J Genzer and R. J Composto
Europhysics Letters (EPL) 38 (3) 171 (1997)
https://doi.org/10.1209/epl/i1997-00221-7

Preparation and Surface Properties of Acrylic Polymers Containing Fluorinated Monomers

Richard R. Thomas, Douglas R. Anton, William F. Graham, et al.
Macromolecules 30 (10) 2883 (1997)
https://doi.org/10.1021/ma9618686

A self-consistent field study of the wetting transition in binary polymer blends

Jan Genzer and Russell J. Composto
The Journal of Chemical Physics 106 (3) 1257 (1997)
https://doi.org/10.1063/1.473222

Comment on “A self-consistent field study of the wetting transition in binary polymer blends” [J. Chem. Phys. 106, 1257 (1997)]

Gerald G. Pereira
The Journal of Chemical Physics 107 (9) 3740 (1997)
https://doi.org/10.1063/1.474731

Thin films of a binary polymer mixture: calculations of the concentration profile for asymmetric walls

C.D Eggleton
Physics Letters A 223 (5) 394 (1996)
https://doi.org/10.1016/S0375-9601(96)00746-3

Wetting transitions in polymer blends: Comparison between simulation and theory

Gerald G. Pereira and Jian-Sheng Wang
The Journal of Chemical Physics 105 (9) 3849 (1996)
https://doi.org/10.1063/1.472205

A self-consistent-field approach to surfaces of compressible polymer blends

F. Schmid
The Journal of Chemical Physics 104 (22) 9191 (1996)
https://doi.org/10.1063/1.471610

Surface enrichment in thin films of PVC and PMMA

K. Kunze, M. Stamm, M. Hartshorne and S. Affrossman
Acta Polymerica 47 (5) 234 (1996)
https://doi.org/10.1002/actp.1996.010470508

Experimental study of surface segregation and wetting in films of a partially miscible polymer blend

M. Geoghegan, R. A. L. Jones, D. S. Sivia, J. Penfold and A. S. Clough
Physical Review E 53 (1) 825 (1996)
https://doi.org/10.1103/PhysRevE.53.825

Evidence for Size Effects on Interfacial Widths in Confined Thin Films

Tobias Kerle, Jacob Klein and Kurt Binder
Physical Review Letters 77 (7) 1318 (1996)
https://doi.org/10.1103/PhysRevLett.77.1318

Analytic theory of surface segregation in compressible polymer blends

Karl F. Freed
The Journal of Chemical Physics 105 (23) 10572 (1996)
https://doi.org/10.1063/1.472944

Concentration profile near the surface of polymer mixtures: a Monte Carlo study

Y. Rouault, B. Dünweg, J. Baschnagel and K. Binder
Polymer 37 (2) 297 (1996)
https://doi.org/10.1016/0032-3861(96)81102-5

Surface phase behavior in binary polymer mixtures. II. Surface enrichment from polyolefin blends

Frank Scheffold, Andrzej Budkowski, Ullrich Steiner, Erika Eiser, Jacob Klein and Lewis J. Fetters
The Journal of Chemical Physics 104 (21) 8795 (1996)
https://doi.org/10.1063/1.471569

Effect of van der Waals surface interactions on wetting transitions in polymer blends

Gerald G. Pereira and Jian-Sheng Wang
Physical Review E 54 (3) 3040 (1996)
https://doi.org/10.1103/PhysRevE.54.3040

Diffusion Limited Wetting

U. Steiner and J. Klein
MRS Proceedings 464 (1996)
https://doi.org/10.1557/PROC-464-121

Interface localization transition in Ising films with competing walls: Ginzburg criterion and crossover scaling

K. Binder, R. Evans, D. P. Landau and A. M. Ferrenberg
Physical Review E 53 (5) 5023 (1996)
https://doi.org/10.1103/PhysRevE.53.5023

Polymer solutions confined in slit-like pores with attractive walls: An off-lattice Monte Carlo study of static properties and chain dynamics

Andrey Milchev and Kurt Binder
Journal of Computer-Aided Materials Design 2 (3) 167 (1996)
https://doi.org/10.1007/BF01198659

Surface Enrichment in a Miscible Polymer Blend: An Experimental Test of Self-Consistent Field and Long-Wavelength Approximation Models

J. Genzer, A. Faldi, R. Oslanec and R. J. Composto
Macromolecules 29 (16) 5438 (1996)
https://doi.org/10.1021/ma951108f

A Monte Carlo study of wetting transitions in polymer blends confined to a capillary

Gerald G. Pereira and Jian-Sheng Wang
The Journal of Chemical Physics 104 (13) 5294 (1996)
https://doi.org/10.1063/1.471258

Phase separation of symmetrical polymer mixtures in thin-film geometry

Y. Rouault, J. Baschnagel and K. Binder
Journal of Statistical Physics 80 (5-6) 1009 (1995)
https://doi.org/10.1007/BF02179862

Surface segregation in blends of styrene-acrylonitrile copolymers

Eugene Kim, Edward J. Kramer, Paul D. Garrett, Robert A. Mendelson and Wan C. Wu
Polymer 36 (12) 2427 (1995)
https://doi.org/10.1016/0032-3861(95)97344-F

A density functional analysis of the effects of surface correlations in simple models of polymer blends

Ka-Yiu Wong, Maria Trache and William E. McMullen
The Journal of Chemical Physics 103 (18) 8257 (1995)
https://doi.org/10.1063/1.470190

Density functionals for polymers near surfaces

William E. McMullen and Maria Trache
The Journal of Chemical Physics 102 (3) 1449 (1995)
https://doi.org/10.1063/1.468877

Influence of conformational asymmetry on the surface enrichment of polymer blends II

James P. Donley and Glenn H. Fredrickson
Journal of Polymer Science Part B: Polymer Physics 33 (9) 1343 (1995)
https://doi.org/10.1002/polb.1995.090330904

Surface effects on polymer blends and block copolymer melts: Theoretical concepts of surface enrichment, surface induced phase separation and ordering

K. Binder
Acta Polymerica 46 (3) 204 (1995)
https://doi.org/10.1002/actp.1995.010460302

Ordering in Macromolecular Systems

Ullrich Steiner, Erika Eiser, Andrzej Budkowski, Lewis Fetters and Jacob Klein
Ordering in Macromolecular Systems 313 (1994)
https://doi.org/10.1007/978-3-642-78893-2_26

The wetting transition for polymer mixtures

R.A.L. Jones
Polymer 35 (10) 2160 (1994)
https://doi.org/10.1016/0032-3861(94)90244-5

Soft Order in Physical Systems

U. Steiner, J. Klein, E. Eiser, A. Budkowski and L. Fetters
NATO ASI Series, Soft Order in Physical Systems 323 133 (1994)
https://doi.org/10.1007/978-1-4615-2458-8_13

Critical point wetting from binary polymer mixtures

Ullrich Steiner, Erika Eiser, Andrzej Budkowski, Lewis Fetters and Jacob Klein
Berichte der Bunsengesellschaft für physikalische Chemie 98 (3) 366 (1994)
https://doi.org/10.1002/bbpc.19940980316

Polymer melt near a solid wall

Pavel K. Brazhnik, Karl F. Freed and Hai Tang
The Journal of Chemical Physics 101 (10) 9143 (1994)
https://doi.org/10.1063/1.468044

Surface studies of polymer blends

E. Occhiello and F. Garbassi
Macromolecular Symposia 78 (1) 131 (1994)
https://doi.org/10.1002/masy.19940780113

Wetting behavior in three‐component polymer blends

R. C. Desai, C. Yeung and J. Noolandi
Acta Polymerica 45 (5) 375 (1994)
https://doi.org/10.1002/actp.1994.010450506

Theories and Mechanism of Phase Transitions, Heterophase Polymerizations, Homopolymerization, Addition Polymerization

K. Binder
Advances in Polymer Science, Theories and Mechanism of Phase Transitions, Heterophase Polymerizations, Homopolymerization, Addition Polymerization 112 181 (1994)
https://doi.org/10.1007/BFb0017984

Self-consistent mean-field calculation of surface segregation in a binary polymer blend

J. Genzer, A. Faldi and R. J. Composto
Physical Review E 50 (3) 2373 (1994)
https://doi.org/10.1103/PhysRevE.50.2373

Phase transitions in thin films of symmetric binary polymer mixtures

Sanat K. Kumar, Hai Tang and Igal Szleifer
Molecular Physics 81 (4) 867 (1994)
https://doi.org/10.1080/00268979400100581

Entropy-driven surface segregation in block copolymer melts

Mohan Sikka, Navjot Singh, Alamgir Karim, et al.
Physical Review Letters 70 (3) 307 (1993)
https://doi.org/10.1103/PhysRevLett.70.307

Reversal of the isotopic effect in the surface behavior of binary polymer blends

Arvind Hariharan, Sanat K. Kumar and Thomas P. Russell
The Journal of Chemical Physics 98 (5) 4163 (1993)
https://doi.org/10.1063/1.465024

Monte Carlo simulation of polymeric materials: Recent progress

K. Binder
Makromolekulare Chemie. Macromolecular Symposia 69 (1) 213 (1993)
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Effect of polymer compatibility on surface enrichment in polymer blends

Panos Sakellariou
Polymer 34 (16) 3408 (1993)
https://doi.org/10.1016/0032-3861(93)90469-Q

Monte Carlo methods for polymer chains in two ‐ dimensional geometries (polymers at surfaces and interfaces)

Kurt Binder
Makromolekulare Chemie. Macromolecular Symposia 65 (1) 175 (1993)
https://doi.org/10.1002/masy.19930650120

The surface composition of miscible polymer blends

R.A.L. Jones and E.J. Kramer
Polymer 34 (1) 115 (1993)
https://doi.org/10.1016/0032-3861(93)90292-I

Free surfaces of polymer blends. I. Theoretical framework and application to symmetric polymer blends

Arvind Hariharan, Sanat K. Kumar and Thomas P. Russell
The Journal of Chemical Physics 98 (8) 6516 (1993)
https://doi.org/10.1063/1.464792

Surface Phase Transition in a Polymer Blend

F Bruder and R Brenn
Europhysics Letters (EPL) 22 (9) 707 (1993)
https://doi.org/10.1209/0295-5075/22/9/012

The effect of finite film thickness on the surface segregation in symmetric binary polymer mixtures

Arvind Hariharan, Sanat K. Kumar, Miriam H. Rafailovich, Jonathan Sokolov, X. Zheng, Daihung Duong, Steven A. Schwarz and Thomas P. Russell
The Journal of Chemical Physics 99 (1) 656 (1993)
https://doi.org/10.1063/1.465738

Free surfaces of polymer blends. II. Effects of molecular weight and applications to asymmetric polymer blends

Arvind Hariharan, Sanat K. Kumar and Thomas P. Russell
The Journal of Chemical Physics 99 (5) 4041 (1993)
https://doi.org/10.1063/1.466100

Surface enrichment in PS/PVME blends: 2. The effect of specific interactions in the bulk mixture

J.M.G. Cowie, B.G. Devlin and I.J. McEwen
Polymer 34 (19) 4130 (1993)
https://doi.org/10.1016/0032-3861(93)90678-4

Comparison of two free-energy expressions and their implications in surface enrichment

Rocco A. Jerry and E. Bruce Nauman
Physical Review E 48 (2) 1583 (1993)
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Surface segregation in a polymer blend. Comparison between Monte Carlo simulation and mean-field theory

P. Cifra, F. Bruder and R. Brenn
The Journal of Chemical Physics 99 (5) 4121 (1993)
https://doi.org/10.1063/1.466108

Effect of long-range forces on surface enrichment in polymer blends

R. A. L. Jones
Physical Review E 47 (2) 1437 (1993)
https://doi.org/10.1103/PhysRevE.47.1437

Spinodal decomposition in thin films of a polymer blend

F. Bruder and R. Brenn
Physical Review Letters 69 (4) 624 (1992)
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Ordering of thin diblock copolymer films

A. Menelle, T. P. Russell, S. H. Anastasiadis, S. K. Satija and C. F. Majkrzak
Physical Review Letters 68 (1) 67 (1992)
https://doi.org/10.1103/PhysRevLett.68.67

Surface tension of random copolymer melts

J. P. Donley and G. H. Fredrickson
Journal of Polymer Science Part B: Polymer Physics 30 (13) 1527 (1992)
https://doi.org/10.1002/polb.1992.090301311

Wetting transitions of asymmetric binary polymer mixtures

Zheng Yu Chen and Jaan Noolandi
Macromolecular Theory and Simulations 1 (1) 31 (1992)
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Chain linear dimensions in the surface‐enriched layer of polymer mixtures

Jian‐Sheng Wang and Kurt Binder
Macromolecular Theory and Simulations 1 (2) 49 (1992)
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Influence of broken conformational symmetry on the surface enrichment of polymer blends

Glenn H. Fredrickson and James P. Donley
The Journal of Chemical Physics 97 (12) 8941 (1992)
https://doi.org/10.1063/1.463969

More insight into critical wetting in polymer blends

Rocco A. Jerry and E. Bruce Nauman
The Journal of Chemical Physics 97 (10) 7829 (1992)
https://doi.org/10.1063/1.463453

The free energy of a binary mixture near a surface with applications to surface enrichment

Rocco A Jerry and E Bruce Nauman
Journal of Colloid and Interface Science 154 (1) 122 (1992)
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X-Ray Evanescent Wave-Induced Fluorescence Study of Polymer Adsorption below the Theta-Point

S. W Barton, L Bosio, R Cortes and F Rondelez
Europhysics Letters (EPL) 17 (5) 401 (1992)
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Model calculations for wetting transitions in polymer mixtures

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